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Jean-Francois Boily Lab

Research group The group investigates how chemical reactions at mineral–water interfaces control key environmental processes, linking molecular-scale mechanisms to large-scale geochemical and climate phenomena. The work follows reactions from single molecules meeting mineral particles to processes spanning entire crystal surfaces.

A central theme is the role of nanometre-thin water and ice films on mineral surfaces. This work challenges the traditional view of ice as chemically inert and shows instead that ice acts as a dynamic geochemical reactor. The group has demonstrated that ice can amplify mineral dissolution, generate reactive species such as Mn(III), and accelerate iron mineral transformations. These findings reshape understanding of weathering in cold environments, including Arctic systems and freeze–thaw cycles.

Scientific focus and climate relevance

The research opens new routes for addressing climate challenges. Studies of CO₂ mineralisation in thin water films show how controlled interfacial processes, including ice formation, can enhance natural weathering and carbon capture, pointing towards scalable mineral-based mitigation strategies. In the Arctic, where rapid warming intensifies freeze–thaw cycles, the same work clarifies how minerals react in thin water and ice films. By showing that ice actively drives dissolution, redox reactions, and the movement of metals and contaminants, it strengthens predictions of effects on water quality and ecosystems in cold regions.

Methods

The group combines experimental and computational techniques to resolve interfacial processes at the molecular level. Spectroscopic tools (FTIR, Raman, sum-frequency generation, XPS) work alongside electrochemical methods (EIS, SECM) to characterise surface reactivity. Molecular simulations (molecular dynamics, density functional theory) extend these measurements into predictive understanding across scales.

Applications and impact

Beyond fundamental discovery, the research supports functional geomaterials for environmental use, including:

  • CO₂ capture and enhanced weathering technologies
  • water treatment and contaminant removal
  • the environmental fate of pollutants and pharmaceuticals
  • the reuse of waste materials as reactive substrates

By joining mechanistic insight with thermodynamic and kinetic modelling, the group turns fundamental science into predictive tools for environmental management, climate mitigation, and sustainable materials design.

 

Read more about the research

 

Publications

Publications

Proceedings of the National Academy of Sciences of the United States of America, Proceedings of the National Academy of Sciences (PNAS) 2026, Vol. 123, (17)
Chen, Tao; Luo, Tao; Bui Thi, Tra My; et al.
Journal of Hazardous Materials, Elsevier 2026, Vol. 504
Bui Thi, Tra My; Chen, Tao; Luo, Tao; et al.
Environmental Science and Technology, American Chemical Society (ACS) 2025, Vol. 59, (46) : 25022-25031
Luo, Tao; Wang, Hao; Chen, Tao; et al.
Geochimica et Cosmochimica Acta, Elsevier 2025, Vol. 406 : 1-4
Boily, Jean-François; Lemke, Kono H.; Stefánsson, Andri
Proceedings of the National Academy of Sciences of the United States of America, Proceedings of the National Academy of Sciences (PNAS) 2025, Vol. 122, (35)
Sebaaly, Angelo P.; van Rijn, Frank; Hanna, Khalil; et al.
Journal of Hazardous Materials, Vol. 493
Bui Thi, Tra My; Chen, Tao; Luo, Tao; et al.
ACS Omega, American Chemical Society (ACS) 2025, Vol. 10, (22) : 22412-22425
Huynh, Chau Minh; Luong, N. Tan; Nguyen, Trung; et al.
Reviews in Mineralogy and Geochemistry, Mineralogical Society of America, Mineralogical Society of America 2025, Vol. 91A, (1) : 105-147
Boily, Jean-François
Physical Chemistry, Chemical Physics - PCCP, Royal Society of Chemistry 2025, Vol. 27, (8) : 4446-4456
Le Crom, Sébastien; Boily, Jean-François
Langmuir, American Chemical Society (ACS) 2025, Vol. 41, (36) : 24336-24343
Chen, Tao; Luo, Tao; Bui Thi, Tra My; et al.
 

Head of research

Overview

Participating departments and units at Umeå University

Department of Chemistry

Research area

Chemical sciences, Materials science

External funding

Swedish Research Council

External funding

En närbild av en snöflinga på en yta.
Ice may release more iron than climate models predict

Most people think of ice as frozen and lifeless, but research at Umeå University shows the opposite.

Ett fruset vattendrag med fjäll i bakgrunden.
Ice dissolves iron faster than liquid water

Arctic rivers are turning rusty orange as permafrost thaws.

Water films – the silent architects of chemical transformations

New chemical knowledge contributes to the fight against global warming and pollution.

Latest update: 2026-06-25